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Extra info for Rarefied gas dynamics : technical papers from the proceedings of the Eighteenth International Symposium on Rarefied Gas Dynamics, University of British Columbia, Vancouver, British Columbia, Canada, July 26-30, 1992
This indicates that CARS is species specific. Figure 3 shows temperature dependence of nitrogen CARS spectra. The spectra are normalized to each principal peak. We observe one strong resonance for the temperature range of 300-1000 K and two strong resonances at higher temperatures. 7 cm'1. 1 cm'1, the rotational structure is not completely resolved. The limitation is based largely on the pump laser linewidth. This effect can be taken into account by convolution of the CARS signal with a slit function.
And Williams, P. , "Resonance Raman Scattering of Light from a Diatomic molecule," Journal of Chemical Physics, Vol. 64, No. 9,1975, pp. 3519-3537. , Murphy, W. , and Bernstein, H. , "Resonance Raman Effect and Resonance Fluorescence in Halogen Gases," Journal of Chemical Physics, Vol. 52, No. 1, 1970, pp. 399^08. McDaniel, J. , "Density Measurement in Compressible Flows Using Off-Resonant Laser Induced Fluorescence," Physics of Fluids, Vol. 25, No. 7,1982, pp. 1105-1107. 11 McClelland, G. , Saenger, K.
Graduate Student, Department of Chemical Engineering. t Professor, Department of Chemical Engineering. 27 28 H. WONGANDJ. R. PERRON coefficients are of special value in the prediction of thermal conductivities of polyatomic mixtures. 5 The main experimental difficulty in Raman spectroscopy is associated with the very weak intensities of the Stokes and antiStokes lines. For this reason, Raman spectroscopy was for sometime confined to liquids and solids which scatter more Raman radiation than gases do.